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Abstract

Nondegenerate two-photon absorption is a nonlinear optical effect in which two photons with different energy are absorbed by a medium simultaneously, resulting in a single electron transition from ground state to excited state through an intermediate virtual state. Compared with the degenerate two-photon absorption coefficient, the absorption coefficient of nondegenerate two-photon absorption is increased by tens or even hundreds of times due to the intermediate resonance effect, so it has great potentials in many nonlinear optical applications. Firstly, the basic principle of two-photon absorption is introduced and the enhancement mechanism of non-degenerate two-photon absorption is explained in this paper. Secondly, the basic method of measuring two-photon absorption is introduced in detail. Thirdly, the reports on nondegenerate two-photon absorption of three-dimensional semiconductor materials and two-dimensional materials are reviewed. Finally, the application progress of infrared detection and imaging, two-photon fluorescence microscope, all-optical switch and optical modulation is summarized, and the future research in this field is summarized and prospected.

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Authors and contacts

Corresponding author:Wu Bo,bowu@m.scnu.edu.cn; Zhou Guo-Fu,guofu.zhou@m.scnu.edu.cn

Funds:Project supported by the National Natural Science Foundation of China (Grant No. 62175068), the Basic and Applied Basic Research Foundation of Guangdong Province, China (Grant No. 2023B1515020024), the Key Laboratory of Optical Information Materials and Technology of Guangdong Province, China (Grant No. 2017B030301007), and the National Green Optoelectronics International Joint Research Center (Grant No. 2016B01018).

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Cited By

DownLoad: Full-Size Img PowerPoint

材料	λ₁/nm	λ₂/nm	β_ND/(cm·GW^–1)	测试条件	β_D/(cm·GW^–1)
CdTe^[34]	870	8840	~1000	10 Hz, 30 ps	~20
ZnS^[34]	~390	~1760	~15	1 kHz, 140 fs	~1
ZnSe^[34]	~480	5600	~270	1 kHz, 140 fs	~2
ZnO^[34]	420	2000	~40	1 kHz, 140 fs	~2.5
GaAs^[34]	870	8840	~800	10 Hz, 30 ps	~10
GaSb^[39]	1720	3550	140	1 kHz, 130 fs	64^[41]
Cu₂O^[42]	800	1494	88	1 kHz, 120 fs	27
MAPbBr₃^[23]	577	1700	53	1 kHz, 100 fs	8^[43]
GaAs/Al_0.32Ga_0.68As QW^[44]	1120	1960	~15	82 MHz, 156 fs	—
WS₂^[45]	620	776	250	80.48 MHz, 250 fs	100
MoSe₂^[45]	790	1500	650	80.48 MHz, 250 fs	80—800
(BA)₂(MA)₃Pb₄X₁₃^[46]	705	760—980	10	100 kHz, 7 fs	—
Si^[40]	1904	1350	0.97	250 kHz, 160 fs	0.5^[47]

DownLoad: CSV

材料	λ₁/nm	λ₂/nm	σ_ND/GM	测试条件	σ_D/GM
罗丹明6 G^[57]	800	691	596	溶剂: 甲醇; 浓度: 16.2 mmol/L; 脉宽: 103 fs	38—150^[58,59]
罗丹明 123^[57]	800	660	776	溶剂: 甲醇; 浓度: 4.2 mmol/L; 脉宽: 103 fs	80^[62]
香豆素6^[57]	800	652	1015	溶剂: 甲醇; 浓度: 23.7 mmol/L; 脉宽: 103 fs	—
香豆素343^[57]	800	651	49	溶剂: 氯仿; 浓度: 27.3 mmol/L; 脉宽: 103 fs	—
尼罗红^[57]	800	669	3270	溶剂: 氯仿; 浓度: 0.75 mmol/L; 脉宽: 103 fs	—
尼罗蓝A^[57]	800	626	1407	溶剂: 氯仿; 浓度: 0.68 mmol/L; 脉宽: 103 fs	—
咔唑衍生物BEMC^[60]	800	650	220	溶剂: 甲醇; 浓度: 10 mmol/L; 脉宽: 140 fs	34
氨基七甲噻吩^[63]	925	1020	1860	溶剂: 甲醇; 浓度: 1.3 mmol/L; 脉宽: 75 fs	940

DownLoad: CSV

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Vol. 72, Issue 20 - 2023-10-20

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