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Abstract

In recent years, organic-inorganic hybrid perovskite solar cells (PSCs) have attracted wide attention due to their high photoelectric conversion efficiency and simple preparation process. Hole transport layer (HTL) is one of the most critical components in PSCs. As a kind of inorganic HTL material, nickel oxide (NiO _x) has been widely used in perovskite solar cells because of its excellent advantages, such as outstanding chemical stability, high carrier mobility, simple methods for its preparation, etc. In this paper, the applications of NiO _xHTL in planar PSCs are systematically summarized from the aspects of the improvment of its structure and photoelectric properties by doping and interface modification. The reasons for affecting the device performances, i.e. fill factor, open-circuit voltage, short-circuit current, photoelectric conversion efficiency, and stability are emphatically analyzed from several aspects, such as energy level matching, hole mobility and crystallinity. In addition, the future development directions of the planar PSCs are prospected.

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Authors and contacts

Corresponding author:Zhang Chen-Xi,zhangchenxi@tyut.edu.cn; Hao Yu-Ying,haoyuying@tyut.edu.cn

Funds:Project supported by the National Natural Science Foundation of China (Grant No. 62074108), the Joint Foundation of National Natural Science Foundation of China and Shanxi Coal-Based Low-Carbon Nurturing Project (Grant No. U1710115), the Major Special Projects of Shanxi Province in Science and Technology, China (Grant No. 20201101012), the Platform and Base Special Project of Shanxi, China (Grant No. 201805D131012-3), and the Natural Science Foundation of Shanxi Province, China (Grant No. 201901D211114)

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Cited By

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器件结构	电压 V_oc/V	电流 J_sc/(mA·cm^–2)	填充因子FF	光电转换效率PCE/%	掺杂/方法	文献
ITO/F2HCNQ:NiO_x/PMMA/CsMAFA/PCBM/BCP/Ag	1.14	23.44	0.83	22.13	F2HCNQ:NiO_xspin-coating	[17]
ITO/F6TCNNQ:NiO_x/CsFAMA/ PCBM/ZrAcac/Ag	1.12	23.18	0.80	20.86	F6TCNNQ/Spin coating	[41]
ITO/Cu:NiO_x/CH₃NH₃PbI₃/C₆₀/BCP/Ag	1.12	22.28	0.81	20.26	Cu:NiO_xNPs/Spin coating	[42]
ITO/Li:Co NiO_x/MA_1yFA_yPbI_3xCl_x/ PCBM/BCP/Ag	1.09	23.80	0.78	20.10	Li:Co/Spin-coating	[40]
ITO/Sr:NiO_x/CH₃NH₃PbI₃/C₆₀/BCP/Ag	1.14	22.66	0.76	19.49	Sr:NiO/Spin-coating	[38]
ITO/NiO_x:AGQDs/CsFAMA/PCBM/BCP/Ag	1.05	22.30	0.83	19.40	NiO_x:AGQDs/Spin-coating	[43]
FTO/Cs:NiO_x/MAPbI₃/PCBM/ZrAcac/Ag	1.12	21.77	0.79	19.35	Cs/Spin coating sol	[37]
ITO/NiMgO/CH₃NH₃PbI₃/PCBM/ZnMgO/Al	1.08	21.30	0.80	18.50	Mg/Sputtering	[44]
FTO/NIR-Co:NiO_x/MAPbI₃/PC₆₁BM/PEI/Ag	1.09	20.46	0.80	17.77	Co/Spin-coating	[35]
FTO/NiMgLiO/MAPbI₃/PCBM/Ti(Nb)O_x/Ag	1.07	20.21	0.75	16.20	Li-Mg/Spray pyrolysis	[45]

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器件结构	电压 V_oc/V	电流 J_sc/(mA·cm^–2)	填充因子FF	光电转换效率PCE/%	改性/方法	文献
ITO/NiO_x/KCl/CsFAMA/PCBM/ZrAcac/Ag	1.15	22.89	0.80	20.96	KCl or NaCl/ Spin-coating	[51]
ITO/NiO_x/PFN-P2/CsFAMA/C₆₀/BCP/Ag	1.13	23.33	0.78	20.50	PFN-P2	[53]
FTO/NiO_x/SDBS/CH₃NH₃PbI₃/ PCBM/BCP/Ag	1.12	22.94	0.78	20.15	SDBS/Spin-coating	[54]
ITO/NiO_x/NH₄F/CH₃NH₃PbI₃/C₆₀/BCP/Ag	1.09	22.45	0.77	18.94	NH₄F/Spin-coating	[50]
ITO/NiO_x/TPI-6MEO/MAPbI₃/ PCBM/BCP/Ag	0.98	23.31	0.81	18.42	TPI-6MEO/ Spin-coating	[49]
ITO/NiO_x/SAM/Perovskite/ PCBM/Bis-C₆₀/Ag	1.11	21.70	0.76	18.40	Benzoic acid modification	[55]
ITO/NiO_x/FDA/CH₃NH₃PbI₃/PCBM/AgAl	1.04	22.55	0.76	17.87	FDA modification	[48]
FTO/NiO_x/PTAA/FA_1–xMA_xPb (I_3–yBr_y)/PCBM/Au	1.06	21.54	0.75	17.10	PTAA/Sol–gel	[56]

DownLoad: CSV

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Vol. 70, Issue 11 - 2021-06-05

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