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Abstract

Polyethylene oxide(PEO) based solid-state batteries have high safety and high energy density, making them suitable for next-generation energy storage devices. However, their energy density reaches a limitation due to the narrow electrochemical window of PEO solid electrolyte. The electrode materials that are compatible with PEO electrolyte is less, thus handering it from being put into wide application. At the PEO/electrode interface, there are side reactions between anode/PEO and PEO cathode. Some strategies are proposed to reduce the side reactions, electrochemical performances of solid-state batteries are improved. To understand the change of interface, several advanced characterizations are employed, which can offer scientific evidence of increasing the interface stability in the future.

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Authors and contacts

Corresponding author:Cong Li-Na,congln816@nenu.edu.cn; Xie Hai-Ming,xiehm136@nenu.edu.cn

Funds:Project supported by the Special Fund of Key Technology Research and Development Projects, China (Grant Nos. 20180201097GX, 20180201099GX, 20180201096GX), the Key Subject Construction of Physical Chemistry of Northeast Normal University, the R&D Program of Power Batteries with Low Temperature and High Energy, the Science and Technology Bureau of Changchun, China (Grant No. 19SS013), the Young Scientists Fund of the National Natural Science Foundation of China (Grant No. 21905041), the Natural Science Foundation of the Education Department of Jilin Province, China (Grant No. JJKH20190265KJ), the Special Foundation of the Industrial Technology Research and Development of Jilin Province, China (Grant No. 2019C042), and the Fundamental Research Funds for the Central Universities (Grant No. 2412020QD006)

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Vol. 69, Issue 22 - 2020-11-20

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