Structure, magnetic and transport properties of Fe<sub>3</sub>O<sub>4</sub> near verwey transition

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Abstract

As the first known metal-insulator transition, Verwey transition of Fe ₃O ₄attracts much attention due to its fascinating physics. With the decreasing temperature across Verwey temperature, Fe ₃O ₄undergoes the transition of lattice distortion, charge ordering, electricity, magnetic anisotropy, etc, but the magnetic ground state keeps the ferrimagnetism. The comprehension of the underlying physics in Verwey transition facilitates the understanding of metal–insulator transition in other strongly-correlated systems. Nevertheless, the mechanism of Verwey transition is still debated after the first glimpse of Verwey transition. In this paper, we summarize the research history and current status of Verwey transition in Fe ₃O ₄. The investigations of lattice structure, charge ordering, electronic transport, magnetic and ferroelectric properties of Fe ₃O ₄across Verwey transition are reviewed. Finally, the summary and outlook are given.

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Corresponding author:Mi Wen-Bo,miwenbo@tju.edu.cn

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交换相互作用	类型和角度	磁性和强度	出现位置
Fe_B-O-Fe_B	超交换, 180°	反铁磁, 强	APB处
Fe_A-O-Fe_A	超交换, 约140°	反铁磁, 强	APB处
Fe_B-O-Fe_A	超交换, 约120°	反铁磁, 强	块体和APB处
Fe_B-O-Fe_B	超交换, 90°	铁磁, 弱	块体和APB处
Fe_A-O-Fe_A	超交换, 约70°	反铁磁, 弱	APB处
Fe_B-Fe_B	直接	铁磁, 弱	块体和APB处
Fe_A-Fe_A	直接	反铁磁, 弱	APB处
Fe_B-Fe_A	直接	铁磁, 弱	APB处

DownLoad: CSV

U/eV	P2/c				$Fd\overline 3 m$
U/eV	↓gap/eV	CS/e	OO(P)	E_t/eV·(f.u.)^–1	↓gap/eV	CS/e	OO(P)	E_t/eV·(f.u.)^–1
0.0	No	0.00	No(0.55)	–0.15	No	0.00	No(0.34)	0.00
4.0	No	0.11	Yes(0.98)	–0.15	No	0.10	Yes(0.96)	–0.22
4.5	0.2	0.15	Yes(0.98)	–0.53	No	0.12	Yes(0.96)	–0.27
5.0	0.42	0.17	Yes(0.97)	–0.75	0.11	0.16	Yes(0.96)	–0.35
5.5	0.63	0.19	Yes(0.96)	–0.85	0.28	0.19	Yes(0.91)	–0.47

DownLoad: CSV

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Vol. 69, Issue 4 - 2020-02-20

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