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Abstract

Infrared spectroscopy can accurately reflect the information of molecular vibration, and it is an important technology to characterize the composition and structure of materials. However, since the interaction between nanomaterials and infrared light is very weak due to the significant size mismatch, it is challenging to obtain the spectral information of nanomaterials in the field of infrared spectroscopy. The plasmon is a collective electron oscillation on the surface of the material inducing by the incident light, and it has excellent light field confinement, which can significantly enhance the interaction between light and nanomaterials. Graphene plasmon has prominent properties, such as high light field confinement, dynamic adjustment, and low intrinsic attenuation. Therefore it is an important solution to enhance the infrared absorption of nanomaterials. This article systematically introduces the infrared plasmon materials system. Then it summarizes the characteristics of graphene plasmon and their advantages on surface enhanced infrared spectroscopy, and it emphasizes the recent important researches and applications of graphene plasmon enhanced infrared spectroscopy in the world, including single molecular layer biochemical detection, gas identification, refractive index sensing, etc. Further prospects for the development and potential applications of graphene plasmon enhanced infrared spectroscopy are also demonstrated.

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Authors and contacts

Corresponding author:Yang Xiao-Xia,yangxx@nanoctr.cn; Dai Qing,daiq@nanoctr.cn

Funds:Project supported by the National Basic Key Research Program of China (Grant No. 2015CB932400), the National Key Research and Development Program of China (Grant No. 2016YFA0201600), the National Natural Science Foundation of China (Grant Nos. 11674073, 11504063, 11704085), the Key Program of the Bureau of Frontier Sciences and Education, Chinese Academy of Sciences (Grant No. QYZDB-SSW-SLH021), the Key Research Program of the Chinese Academy of Sciences (Grant No. ZDBS-SSW-JSC002), and the Youth Innovation Promotion Association Chinese Academy of Sciences and CAS Interdisciplinary Innovation Team (Grant No. JCTD-2018-03).

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红外表面等离激元材料	载流子迁移率cm²/(V·s)	可调性	局域能力λ_IR/λ_p	品质因子
金属(如Au, Ag)^[31,32]	～10⁰—10^{2 [33]}	电学不可调	< 5^[34]	< 36^[30]
半导体(如Ge, ITO)^[35,36]	～10⁰—10^3[36]	电学可调	< 10^[30]	< 37^[30]
超导体(如FeSe)^[37,38]	～10^4[39]*	电学可调	—	—
拓扑绝缘体(如Bi₂Se₃)^[40,41]	～10^4[42]	电学可调	< 900^[41,43]	3^[43]
石墨烯^[30,31]	～10³—10^5[30]	电学可调	～40—220^{[7,18,30,34,43]}	< 130*^[30]
碳纳米管^[44,45]	～10³—10^{4 [46]}	电学可调	～100—1000^[47]	< 26^[47,48]
注: *表示低温.

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石墨烯等离激元
等离激元响应波段	近红外(0.7—2.5 μm)	中红外(2.5—25 μm)	远红外及太赫兹(> 25 μm)
能否激发	否	能	能
尺寸	—	～100 nm	～1 μm
本征寿命	—	～20—120 ps^a	～0—40 ns^a
局域能力	—	～40—220^b	< 50^c
注: a摘自文献[74]; b摘自文献[7,17,43]; c摘自文献[76,77].

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Vol. 68, Issue 14 - 2019-07-20

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