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Abstract

Photovoltaic technology, which can converse solar illumination into electricity, is crucial to the sustainable development of human civilization. Among them, the organic-inorganic hybrid perovskite solar cell (OIPSC) has become a research front due to its excellent photoelectric characteristics, low production cost and high power conversion efficiency (PCE). Although the PCE of OIPSC has exceeded 24%, the organic components in the perovskite system are sensitive to the decomposion caused by either being exposed to light or heated in high temperature environment. The stability defects have greatly limited the commercialization of perovskite solar cells. Therefore, it is urgent to improve the stability of perovskite solar cells, especially to solve the material decomposition problem. All-inorganic perovskite photovoltaic material, composed of all-inorganic elements, exhibits excellent heat and moisture resistance. Therefore, the development of all-inorganic perovskite solar cells is of great significance for solving the current stability problems in perovskite photovoltaics. In this work, we review the recent research progress of all-inorganic perovskite solar cells, discuss the solution approaches to processing all-inorganic perovskite films, and explore the enhancement of device stability. Our work provides a guideline for further promoting the device stability and PCE.

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Authors and contacts

Corresponding author:Liu Peng-Yi,tlpy@jnu.edu.cn; Zheng Yi-Fan,yifan.zheng@pku.edu.cn;

Funds:Project supported by the National Natural Science Foundation of China (Grant Nos. 11804117, 61674070), the Fundamental Research Funds for the Central Universities, China (Grant No. 21618313), the Key Science and Technology Program of Guangdong Province, China (Grant No. 2017B09090701), and the China Postdoctoral Innovation Talent Foundation (Grant No. 8206200013).

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Cited By

DownLoad: Full-Size Img PowerPoint

电池结构	制备方法	V_OC/V	J_sc/mA·cm^–2	FF/%	PCE/%	参考文献
FTO/PEDOT:PSS/CsPbI₃/PCBM/Al	溶液法	~0.9	3		1.7	[26]
FTO/c-TiO₂/CsPbI₃/Spiro-OMeTAD/Au	溶液法	0.8	12		2.9	[26]
FTO/c-TiO₂/m-TiO₂/CsPbI₃/Spiro-OMeTAD/Au	溶液法	~0.6	8		1.3	[26]
FTO/c-TiO₂/CsPbI₃/CuI/Au	溶液法	0.89	16.02	56.59	8.07	[149]
FTO/c-TiO₂/CsPb_0.96Bi_0.04I₃/CuI/Au	溶液法	0.97	18.76	72.59	13.21	[149]
FTO/TiO₂/CsPbI₃/Spiro-OMeTAD/Ag	溶液法	0.66	11.92	52.47	4.13	[39]
FTO/c-TiO₂/CsPbI₃/Carbon	溶液法	0.67	14.31	48	4.65	[38]
FTO/c-TiO₂/m-TiO₂/CsPbI₃/Carbon	溶液法	0.58	13.74	44	3.48	[38]
FTO/TiO₂/AX-coatedCsPbI₃-QDs/Spiro-OMeTAD/MoO_x/Al	溶液法	1.16	15.24	76.63	13.43	[110]
FTO/TiO₂/CsPbI₃QDs/Spiro-OMeTAD/MoO_x/Al	溶液法	1.23	13.47	65	10.77	[23]
MgF₂/FTO/c-TiO₂/m-TiO₂/CsPb_0.95Ca_0.05I₃/P3HT/Au	溶液法	0.95	17.9	80	13.5	[78]
ITO/PTAA/zwitterion-CsPb(I_0.98Cl_0.02)₃/PCBM/C₆₀/BCP/Al	溶液法	1.09	14.9	70	11.4	[150]
ITO/TiO₂/CsPbBr₃/Carbon	溶液法	0.64	5.3	64	3.9	[151]
FTO/TiO₂/CsPbI₂Br-0.02MnCl₂/PCBM/Ag	溶液法	1.172	14.37	80	13.47	[85]
FTO/TiO₂/CsPbI₂Br/PTAA/Au	溶液法	1.177	14.25	80.2	13.45	[77]
FTO/TiO₂/CsPbI₃QDs/PTAA/Au	溶液法	1.192	11.75	78.3	10.97	[77]
FTO/c-TiO₂/CsPbI₃-0.05DETAI₃/P3HT/Au	溶液法	1.06	12.21	61	7.89	[101]
FTO/TiO₂/quasi-2D Cs_0.9PEA_0.1PbI₃/Spiro-OMeTAD/Au	溶液法	0.838	10.96	62	5.7	[128]
FTO/NiO_x/InCl₃:CsPbI₂Br/ZnO@C₆₀/Ag	溶液法	1.15	15.1	78	13.57	[91]
FTO/NiO_x/CsPbI₂Br/ZnO@C₆₀/Ag	溶液法	1.1	15.1	78	12.92	[91]
FTO/TiO₂/CsPbI₃/Carbon	溶液法	0.79	18.5	65	9.5	[37]
FTO/TiO₂/CsPbI₃QDs/PTB7/MoO_x/Ag	溶液法	1.27	12.39	80	12.55	[112]
FTO/c-TiO₂/BA₂CsPb₂I₇/Spiro-OMeTAD/Au	溶液法	0.957	8.88	57	4.84	[127]
FTO/TiO₂/CsPb_0.995Mn_0.005I_1.01Br_1.99/Carbon	溶液法	0.99	13.15	57	7.36	[86]
FTO/bl-TiO₂/2 wt% Sn-TiO₂/Cs₂SnI₄Br₂/solid state Cs₂SnI₆based HTM/LPAH	溶液法	0.563	6.22	57.7	2.025	[52]
FTO/TiO₂/CsPbI₂Br/CsPbI₃QDs/PTAA/Au	溶液法	1.204	15.25	78.7	14.45	[77]
FTO/c-TiO₂/m-TiO₂/CsPbBr₃/MoS₂QDs/Carbon	喷涂法	1.307	6.55	79.4	6.80	[152]
FTO/c-TiO₂/m-TiO₂/CsPbIBr₂/Spiro-OMeTAD/Au	喷涂法	1.121	7.9	70	6.2	[59]
FTO/SnO₂QDs/CsPbBr₃/carbon	溶液法	1.572	7.68	75	9.15	[50]
ITO/PEDOT:PSS/CsPbBr₃/PCBM/Ag	溶液法	0.982	5.9	73.7	4.5	[135]
FTO/m-TiO₂/CsPbBr₃/CsBi_2/3Br₃/carbon	溶液法	1.594	7.75	80.9	10.0	[50]
FTO/SnO₂QDs/CsPbBr₃/CsSnBr₃QDs/carbon	溶液法	1.610	7.8	84.4	10.6	[50]
FTO/m-TiO₂/Cs₂AgBiBr₆/Spiro-MeOTAD/Ag	溶液法	0.98	3.93	63	2.43	[76]
FTO/TiO₂/PTABrCsPbI₃/Spiro-MeOTAD/Ag	溶液法	1.104	19.15	68.5	17.06	[27]
FTO/TiO₂/CsPbI₃/Spiro-MeOTAD/Ag	溶液法	1.051	18.89	68.5	13.61	[27]
PET/ITO/TiO₂/CsPb_0.96Bi_0.04I₃/Spiro-OMeTAD/Au	溶液-气相辅助法	1.05	15.11	72.32	11.47	[87]
ITO/TiO₂/CsPbI₃/P3HT/Au	气相法	1.063	13.8	71.6	10.5	[142]
ITO/TiO₂/CsPbI₃/Au	气相法	0.959	8.7	56	4.7	[46]
ITO/C₆₀/CsPbI₂Br/TAPC/MoO₃/Ag	气相法	1.15	15.2	67	11.7	[140]
FTO/TiO₂/CsPbI₃/P3HT/Ag	气相法	0.79	12..06	72	6.79	[146]

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Vol. 68, Issue 15 - 2019-08-05

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