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摘要

基于超快强激光与物质相互作用的高次谐波产生(high-order harmonic generation, HHG)提供了非微扰区光与物质相互作用的研究平台, 同时也是台式化极紫外光源和阿秒脉冲的主要产生途径. 非微扰区固体HHG涉及超快强场物理、凝聚态物理、材料科学和信息科学等领域的核心内容, 自2011年首次在实验中观察到以来, 迅速成为强场物理和阿秒科学的研究前沿. 本综述从一个实验工作者的角度, 总结了固体HHG的研究进展和重要应用. 首先通过对比高次谐波(high-order harmonic, HH)产率和截止能量对驱动激光参数的依赖关系, 展示固体HHG与气体HHG截然不同的特性. 重点介绍固体HHG调控和应用方面的进展, 包括通过设计靶材结构或者激光光场实现对HH产率、偏振、时空分布等精密调控, 以及固体HH谱学技术在材料结构表征和超快电子动力学研究等领域的应用. 最后对固体HHG的未来发展进行了展望.

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Abstract

The generation of high-order harmonics based on the interaction between ultrafast intense laser and matter provides a platform for studying the light-matter interaction in the non-perturbative region. It is also the main route to generating desktop extreme ultraviolet light source and attosecond pulse. The non-perturbative solid high-order harmonic involves the core content of ultrafast strong field physics, condensed matter physics, materials science, information science and other fields. Since it was first experimentally observed in 2011, it has rapidly become the research frontier of strong field physics and attosecond science. This review summarizes the research progress and important applications of solid high-order harmonics from the perspective of an experimentalist. Firstly, distinct characteristics are shown for solid high-order harmonic by comparing the dependence of harmonic yield and cut-off energy on driving laser parameters with gas high-order harmonic. Then, the progress of manipulation and application are highlighted for solid high-order harmonic, including the precise control of harmonic yield, polarization, space-time distribution through the design of target structure or laser field, as well as the application of solid high-order harmonic spectroscopy in the fields of material structure characterization and ultrafast electron dynamics. Finally, the future is prospected for the study of solid high-order harmonics.

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作者及机构信息

通信作者:吴成印,cywu@pku.edu.cn

基金项目:国家重点研发计划(批准号: 2018YFA0306302)和国家自然科学基金(批准号: 12174011, 11625414)资助的课题.

Authors and contacts

Corresponding author:Wu Cheng-Yin,cywu@pku.edu.cn

Funds:Project supported by the National Key R&D Program of China (Grant No. 2018YFA0306302) and the National Natural Science Foundation of China (Grant Nos. 12174011, 11625414).

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施引文献

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