This paper reports the generation of the coherent and stimulated radiation in UV, visible and infrared regions by two-photon pumping. It includes the tunable coherent radiation around 1.03 μm generated by a special six-wave mixing process, the stimulated radiation at 812.6 nm generated by molecular two-photon dissociation or atomic cascade transition, coherent radiation at 323.3 nm and 670.8 nm generated by the four-wave mixings.