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摘要

当今世界能源浪费巨大, 其中绝大多数以废热的形式被浪费掉. 热电效应可以将热能转换为电能并且没有危险物质的释放, 因此热电效应的应用吸引了越来越多人的兴趣. 自从石墨烯被发现以来, 越来越多的二维层状材料被报道, 它们通常比体块材料有着更加优越的电学、光学等物理性质, 而新的理论和实验技术的发展, 也促进了人们对于它们的研究. 在本文中, 首先介绍了基于二维材料热电性质的测量方法和测试技术, 并对其测试中具有挑战性的问题进行讨论. 随后对石墨烯、过渡金属硫化物、黑磷等材料的热电应用进行了介绍. 最后, 讨论了提升热电性能的各种策略与亟待解决的问题, 并对此做出展望.

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Abstract

Nowadays, there are enormous amounts of energy wasted in the world, most of which is in the form of wasted heat. Thermoelectric effect, by converting heat energy into electricity without releasing dangerous substances, has aroused more and more interest from researchers. Since the discovery of graphene, more and more two-dimensional layered materials have been reported, which typically own superior electrical, optical and other physical properties over the bulk materials, and the development of the new theory and experimental technologies stimulates further research for them as well. In this work, first we introduce the measurement methods and techniques that are suitable for characterizing the thermoelectric properties of two-dimensional materials, and then discuss the relevant current challenging issues. Subsequently, graphene, transition metal disulfides, black phosphorus and other 2-dimensional materials in thermoelectric applications are introduced. Finally, we discuss the various strategies to improve the thermoelectric performance and the problems that need solving urgently.

Keywords:

作者及机构信息

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通信作者:张力发,phyzlf@njnu.edu.cn; 吴靖,wujing@imre.a-star.edu.sg; 赵云山,phyzys@njnu.edu.cn

基金项目:国家自然科学基金(批准号: 12204244)、江苏省自然科学基金(批准号: BK20210556)和江苏省特聘教授项目资助的课题

Authors and contacts

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Corresponding author:Zhang Li-Fa,phyzlf@njnu.edu.cn; Wu Jing,wujing@imre.a-star.edu.sg; Zhao Yun-Shan,phyzys@njnu.edu.cn

Funds:Project supported by the National Natural Science Foundation of China (Grant No. 12204244), the Natural Science Foundation of Jiangsu Province, China (Grant No. BK20210556), and the Jiangsu Specially-Appointed Professor Program, China.

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参考文献

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施引文献

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

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