As an important optical element of the optical integration in the future, nanolasers has been a research hotspot in recent years, and the corresponding structural engineering and output characteristics have been widely investigated. However, the nonlinear dynamical performances of nanolasers are rarely reported. Only some preliminary analyses of the dynamic behavior under the optical feedback, optical injection and mutual injection can be found. Some researches pointed out the future prospect of nanolasers, however, some chaos-based applications have not been explored. Therefore, we numerically investigate chaos dynamics in a nanolaser subjected to optical feedback and in another nanolaser subjected to chaotic injection from the former structure by using single mode rate equation, which includes the Purcell cavity-enhanced spontaneous emission factor Fand spontaneous emission coupling factor β. The Fdenotes the ratio of the spontaneous emission rate into the cavity mode to the total spontaneous emission rate in the bulk medium in the absence of a cavity and βrepresents the fraction of spontaneous emitted photons which are coupled into cavity mode. Specifically, chaos time delay signature (TDS) and unpredictability are evaluated by the peak size of autocorrelation function (ACF) and permutation entropy (PE) respectively. Such kinds of calculations have the advantage of fast operation speed and anti-noise robustness. The results show that the increasing of bias current and the decreasing of gain saturation factor ε, Fand βare beneficial to improving the unpredictability and suppressing TDS because the weak damping of the relaxation oscillation leads to strong oscillation. Large linewidth enhancement factor αwill increase the number of laser oscillating modes, sideband modes, the spectral components, and enhance the dispersion effect, which will also weaken the information about outer cavity and improve the complexity of chaos. In addition, the above-mentioned chaos properties can be enhanced by injecting the chaos output from a nanolaser subjected to optical feedback into another (slave) nanolaser, which is due to the nonlinear interaction between the driving chaotic signal and the internal electric field of the slave nanolaser. Finally, two-dimensional maps depicting high unpredictability and TDS concealment in the parameter space of the frequency detuning and the injection strength are obtained. It can be found that unpredictability degree can be enhanced by choosing high detuning frequency and intermediate injection strength in the non-injection locking area. The numerical results pave the way for generating the high-quality chaotic sources on a chip or the photonic integrated circuits based on novel semiconductor nanolaser and its related applications.