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摘要

等离激元共振能量转移指表面等离激元将俘获的能量通过偶极-偶极相互作用转移到邻近的半导体或分子等激子体系中, 它是等离激元非辐射弛豫的一个通道, 也可作为获取和利用等离激元共振能量的一种方式. 此外, 等离激元能量还可以通过热电子弛豫(非辐射)和光散射(辐射)等方式耗散. 等离激元各个弛豫通道之间存在着很强的关联, 相关的能量转移和电荷转移过程可以将等离激元耗散的能量输送到其他体系或转换为其他能量形式. 本文主要介绍了等离激元共振能量转移和与其相关的能量和电荷转移过程(包括等离激元近场增强及耦合、远场散射、热电子弛豫等)的物理机制和动力学性质, 并详细介绍了这些机制在增强光催化研究领域的最新进展.

关键词:

Abstract

Plasmon resonance energy transfer refers to the coherent energy transfer via dipole-dipole coupling from surface plasmons to adjacent exciton nanosystems such as semiconductor quantum dots or dye molecules. The plasmon resonance energy transfer is a non-radiative plasmon decay pathway, which can also act as an available channel to extract the plasmon-harvested energy. In addition, hot electron relaxation (non-radiative channel) and scattering (radiative channel) are also the dissipation pathways of surface plasmon resonances. The plasmon-harvested energy can be effectively transferred to other nanosystems or converted into other energy forms through these correlated dissipation pathways. In this paper, the underlying mechanism and dynamics of the plasmon resonance energy transfer as well as the related energy and charge transfer processes (such as near field enhancement and coupling, far field scattering, plasmon-induced hot electron transfer) are introduced. The recent research progress of the plasmon-enhanced photocatalysis by energy and charge transfer is reviewed.

Keywords:

作者及机构信息

周利^1,2,
王取泉^1,3

1.
2.
3.

通信作者:王取泉,qqwang@whu.edu.cn

基金项目:国家重点研发计划(批准号: 2017YFA0303402)、国家自然科学基金(批准号: 11874293, 91750113, 11674254)、湖北省自然科学基金(批准号: 2018CFB572)和武汉大学基金资助的课题.

Authors and contacts

Zhou Li^1,2,
Wang Qu-Quan^1,3

1.
2.
3.

Corresponding author:Wang Qu-Quan,qqwang@whu.edu.cn

Funds:Project supported by the National Key Research and Development Program of China (Grant No. 2017YFA0303402), the National Natural Science Foundation of China (Grant Nos. 11874293, 91750113, 11674254), the Hubei Provincial Natural Science Foundation of China (Grant No. 2018CFB572), and the Young Talent Training Program of Wuhan University, China.

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施引文献

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

下载: 全尺寸图片幻灯片

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